I can't authenticate my old steam account in order to unlink, and then update, the cross-save setup with my new steam account (old account requested closed because I could no longer access an old school email). Can I simply have this old account removed so that I can unlink and update my accounts? I have no way to send an email to support to help me on this but nothing else I have tried to get access to the old account works.
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If that old account is deleted then you are stuck that way. Nothing can be done to remove it.