The worst ragequit I've ever had had to be in NBA 2K13, during Game 7 of the NBA Finals. It was nearing the end of the first half and my player had managed to stock up about 5 fouls before the 2 minute mark. Just as the half was about to finish, I fouled out. I could've cost our team the game had I not quit the current session and reloaded later on. But that still didn't stop me from breaking my controller, punching the shit out of my TV, and nearly breaking my wrist while trying to punch a wall. I got to say, I've honestly raged more at 2K than I ever have at Call Of Duty or any other game. Kind of surprising...
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I was like 13, playing New Super Mario Bros for the DS. I couldn't beat the first world, probably deleted and restarted my file two times out of frustration. I died while fighting the first boss at the end for the millionth time and threw my DS, gave the game to my little sister (who beat the game in a few weeks) and have never played a single platforming game since.