In my opinion, Halo 2 is still the best Halo game.
Explorability, replayability, and a fantastic mutliplayer experience. Not just competitively, but in a social way too. Superbounces everywhere, out of maps and various other glitches were part of what made Halo 2 so amazing.
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The game was rife with glitches and cheaters, though multiplayer was superb and is what got me addicted to Xbox LIVE. Halo 3 was a much more perfected experience. That was the game I spent all work looking forward to getting home and playing every night.