I do love Knucklehead but the More Super From Killing Enemies is also a perk for the Raid helmet. And if you use the Raid Helmet with Young Ahamkara's Spine you also get more Super Energy from grenade kills which seems like the best overall setup. So basically the Raid helmet currently is the best helmet because it not only gives you more super from kills but also opens a slot to get more super from grenades as well.
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good thinking! Maybe I am too used to have the Radar up all the time ;-)