Well, a couple....
1.) Deus Ex: Human Revolution- first time I stabbed someone with my elbow-mounted, spring loaded arm katanas.
2.) Fallout 3- First time I saw Washington D.C., and the Washington Monument with a huge chunk out of the side.
3.) Mass Effect 2- The assault on the Collector Base- when you fly up to the collector base, and get shot at, I had bought all of the Upgrades, so the crew were all saying things along the lines of 'Good thing we got the extra armour!' Etc.
English
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I just got Fallout 3 back today. Gonna give it another go.
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Yeah, I had been thinking about buying it for a long time, and finally got it at a sale- one of the best decisions of my life...