I currently have a couple of gauntlets and an artifact that's a higher light level than my equipped legendaries, but it's NOT possible to use these for infusion. Legendary artifact is at 287 -> Rare artifact at 299 - NOT possible to infuse legendary with this one. I have encountered this several times w/gauntlets, boots and artifacts! Hey... What is the dealio?
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It should work if you've the necessary materials, the gear isn't locked and the stuff you're dismantling isn't equipped. You get a message come up anyway so what does it say?