Right now i have all legendary armor that can obtain 33 light. Is it best for me now to use some Vanguard marks to buy some resources or is it better to save them and just go find them in the patrol missions.
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Well if you have patience, then do patrol, if you want it badly, then buy it
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This is all dependent on how often you play; doing raids and strike playlists. I would say if you plan on doing Crota, and you are high enough level, strive to get those armor pieces and spend the marks on upgrading that. If you play a lot and get marks quickly, then go ahead and buy the resources because it's a very efficient way of getting them. I hope I helped a little!
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Up to you. I personally don't use marks for materials, so long as I have a need for marks otherwise. Remember that one use is to buy armor and break it down for ascendant shards. But if you have all the armor, weapons, and ascendants you need to power them up (from the tower vendor appropriate to your mark), usin marks to buy mats can save a lot of time. Be sure to run the daily heroic and the daily patrol bounty, for some extra mats, also.